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鍥?/span>1. TDI鍒?/span>瀛?/span>緇?/span>鏋?/span>鍙?/span>鍏?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鍜?/span>姘?/span>閿?/span>鍝?/span>搴?/span>紺?/span>鎰?/span>鍥?/span>


浠?/span>浠?/span>鍦?/span>鐮?/span>絀?/span>榪?/span>紼?/span>涓?/span>鍋?/span>鐒?/span>鍙?/span>鐜?/span>錛?/span>闅?/span>鐫姘?/span>鐨?/span>閫?/span>娓?/span>鍔?/span>鍏?/span>錛?/span>TDI鐨?/span>鍥?/span>姘?/span>鍛?/span>鍠?/span>婧?/span>娑?/span>鐨?/span>鑽?/span>鍏?/span>棰?/span>鑹?/span>閫?/span>娓?/span>浠?/span>钃?/span>鑹?/span>鍙?/span>涓?/span>闈?/span>鑹?/span>銆?/span>鍏?/span>鑽?/span>鍏?/span>鍙?/span>灝?/span>寮?/span>搴?/span>鏈?/span>鐫鏄?/span>钁?/span>鐨?/span>澧?/span>寮?/span>錛?/span>鍥?/span>2錛?/span>銆?/span>鍥?/span>涓?/span>娌?/span>鏈?/span>鑱?/span>闆?/span>浣?/span>鐨?/span>褰?/span>鎴?/span>錛?/span>鎵浠?/span>鍙?/span>浠?/span>鎺?/span>闄?/span>鎺?/span>鑱?/span>闆?/span>璇?/span>瀵?/span>鍙?/span>鍏?/span>錛?/span>AIE錛?/span>鏈?/span>鐞?/span>瀵?/span>鑷?/span>鐨?/span>鑽?/span>鍏?/span>澧?/span>寮?/span>鐜?/span>璞?/span>銆?/span>鑰?/span>嬋鍙?/span>鍏?/span>璋?/span>鍜?/span>鍙?/span>灝?/span>鍏?/span>璋?/span>鐨?/span>閲?/span>鍙?/span>鍙?/span>浠?/span>鎺?/span>闄?/span>寮?/span>鏋?/span>鍖?/span>錛?/span>鐑?/span>閱?/span>寮?/span>寮?/span>鏋?/span>鍖?/span>錛?/span>瀵?/span>鑷?/span>鐨?/span>榪?/span>涓鐜?/span>璞?/span>銆?/span>


鍥?/span>2. TDI鍦?/span>涓?/span>鍚?/span>姘?/span>鍚?/span>閲?/span>鐨?/span>鍥?/span>姘?/span>鍛?/span>鍠?/span>婧?/span>娑?/span>涓?/span>鐨?/span>鍚?/span>鏀?/span>銆?/span>鍙?/span>灝?/span>鍜?/span>嬋鍙?/span>鍏?/span>璋?/span>


闄?/span>浜?/span>AIE鏈?/span>鐞?/span>涔?/span>澶?/span>錛?/span>婧?/span>鍓?/span>鏋?/span>鎬?/span>鍙?/span>鍖?/span>鍜?/span>姘?/span>閿?/span>浣?/span>鐢?/span>鏄?/span>鍙?/span>澶?/span>涓?/span>涓?/span>鍙?/span>鑳?/span>瀵?/span>鑷?/span>榪?/span>涓鍙?/span>鍏?/span>綰?/span>縐?/span>鍜?/span>澧?/span>寮?/span>鐜?/span>璞?/span>鐨?/span>鍙?/span>鑳?/span>鍘?/span>鍥?/span>銆?/span>鍥?/span>姝?/span>錛?/span>鐮?/span>絀?/span>浜?/span>鍛?/span>嫻?/span>璇?/span>浜?/span>TDI鍦?/span>涓?/span>鍚?/span>鏋?/span>鎬?/span>婧?/span>鍓?/span>涓?/span>鐨?/span>鍏?/span>璋?/span>銆?/span>濡?/span>鍥?/span>3鎵紺?/span>錛?/span>TDI鍦?/span>浜?/span>姘?/span>鐢?/span>鐑?/span>銆?/span>鐢?/span>鑻?/span>銆?/span>涔?/span>鑵?/span>銆?/span>N,N-浜?/span>鐢?/span>鍩?/span>鐢?/span>閰?/span>鑳?/span>絳?/span>涓?/span>鍚?/span>鏋?/span>鎬?/span>鐨?/span>闈?/span>璐?/span>瀛?/span>婧?/span>鍓?/span>涓?/span>鏈?/span>鐫鐩?/span>浼?/span>鐨?/span>鍙?/span>灝?/span>錛?/span>鍏?/span>鏈澶?/span>鍙?/span>灝?/span>娉?/span>闀?/span>鍧?/span>鍦?/span>425 nm宸?/span>鍙?/span>銆?/span>鑰?/span>鍦?/span>鐢?/span>閱?/span>銆?/span>涔?/span>閱?/span>鎴?/span>鑰?/span>涓?/span>閱?/span>絳?/span>璐?/span>瀛?/span>婧?/span>鍓?/span>涓?/span>錛?/span>TDI鐨?/span>鏈澶?/span>鍙?/span>灝?/span>娉?/span>闀?/span>綰?/span>縐?/span>鑷?/span>470 nm宸?/span>鍙?/span>錛?/span>騫?/span>涓?/span>鍙?/span>鍏?/span>寮?/span>搴?/span>鏈?/span>鐫鏄?/span>钁?/span>鐨?/span>澧?/span>寮?/span>銆?/span>榪?/span>琛?/span>鏄?/span>姘?/span>閿?/span>浣?/span>鐢?/span>鍙?/span>鑳?/span>鏄?/span>鑽?/span>鍏?/span>澧?/span>寮?/span>鐨?/span>鍘?/span>鍥?/span>銆?/span>


鐞?/span>璁?/span>璁?/span>綆?/span>緇?/span>鏋?/span>琛?/span>鏄?/span>錛?/span>TDI鐨?/span>鑽?/span>鍏?/span>鍙?/span>灝?/span>鎬?/span>鏄?/span>錛?/span>蟺*鈫?/span>蟺錛?/span>灞?/span>鎬?/span>鐨?/span>LUMO鈫?/span>HOMO璺?/span>榪?/span>銆?/span>鑰?/span>S2鈫?/span>S0鏄?/span>錛?/span>蟺*鈫?/span>n錛?/span>灞?/span>鎬?/span>LUMO鈫?/span>HOMO-1璺?/span>榪?/span>銆?/span>鍓?/span>浜?/span>鐨?/span>鐮?/span>絀?/span>琛?/span>鏄?/span>錛?/span>n杞?/span>閬?/span>鐨?/span>鑳?/span>綰?/span>瀹?/span>鏄?/span>鍙?/span>鍒?/span>姘?/span>閿?/span>鐨?/span>褰?/span>鍝?/span>銆?/span>鍦?/span>姘?/span>閿?/span>鐨?/span>浣?/span>鐢?/span>涓?/span>錛?/span>n杞?/span>閬?/span>鐨?/span>鑳?/span>綰?/span>浼?/span>閫?/span>娓?/span>涓?/span>鍗?/span>錛?/span>浠?/span>鑰?/span>瀵?/span>鑷?/span>鍘?/span>鏈?/span>鐨?/span>LUMO鈫?/span>HOMO-1璺?/span>榪?/span>鍙?/span>涓?/span>鑽?/span>鍏?/span>鍙?/span>灝?/span>鎬?/span>銆?/span>榪?/span>鍙?/span>鑳?/span>鏄?/span>TDI鍒?/span>瀛?/span>鍦?/span>璐?/span>瀛?/span>婧?/span>鍓?/span>涓?/span>鍙?/span>灝?/span>綰?/span>縐?/span>鐨?/span>鍘?/span>鍥?/span>銆?/span>


鍥?/span>3. TDI鍦?/span>涓?/span>鍚?/span>婧?/span>鍓?/span>涓?/span>鐨?/span>鍏?/span>璋?/span>鍜?/span>鍙?/span>鑳?/span>鐨?/span>鍙?/span>鍏?/span>鏈?/span>鐞?/span>紺?/span>鎰?/span>鍥?/span>


浠?/span>浠?/span>鍦?/span>鐢?/span>閲?/span>灞?/span>鍕?/span>鎴?/span>鑰?/span>鐜?/span>鐠?/span>媯?/span>鍒?/span>TDI鐨?/span>鍗?/span>鏅?/span>鏃?/span>錛?/span>鍙?/span>浠?/span>鍙?/span>鐜?/span>鏄?/span>浜?/span>鐨?/span>鍙?/span>鍏?/span>銆?/span>榪?/span>涓鏄?/span>浜?/span>鐨?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>瀵?/span>浜?/span>綰?/span>鏈?/span>鏈?/span>鏉?/span>鏂?/span>鏉?/span>璇?/span>鏄?/span>杈?/span>涓?/span>闅?/span>寰?/span>鐨?/span>銆?/span>鍒?/span>鐢?/span>鍏?/span>綰?/span>鍏?/span>璋?/span>浠?/span>閲?/span>闆?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鐨?/span>鍏?/span>璋?/span>鍙?/span>鐜?/span>鍏?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鍏?/span>璋?/span>鍜?/span>鍏?/span>鑷?/span>鍙?/span>鍏?/span>涓?/span>涓鑷?/span>銆?/span>榪?/span>涓鐜?/span>璞?/span>鍙?/span>鑳?/span>鏄?/span>鐢?/span>浜?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鍜?/span>鍏?/span>鑷?/span>鍙?/span>鍏?/span>鏄?/span>涓?/span>縐?/span>涓?/span>鍚?/span>鐨?/span>鍙?/span>鍏?/span>瀵?/span>鑷?/span>鐨?/span>銆?/span>鍗?/span>鏅?/span>琛?/span>灝?/span>瀹?/span>楠?/span>琛?/span>鏄?/span>錛?/span>鍦?/span>TDI鐨?/span>鏅?/span>浣?/span>涓?/span>錛?/span>TDI鍒?/span>瀛?/span>鏄?/span>浜?/span>閿?/span>鎺?/span>鍒?/span>鐨?/span>銆?/span>榪?/span>縐?/span>浜?/span>閿?/span>鎺?/span>鍒?/span>鍙?/span>鑳?/span>鏄?/span>璇?/span>鏅?/span>浣?/span>鏈?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鐜?/span>璞?/span>鐨?/span>鍏?/span>閿?/span>銆?/span>


鍥?/span>4. TDI鏅?/span>浣?/span>鐨?/span>鍚?/span>鏀?/span>鍏?/span>璋?/span>銆?/span>鑽?/span>鍏?/span>鍏?/span>璋?/span>銆?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鍏?/span>璋?/span>鍜?/span>鍗?/span>鏅?/span>緇?/span>鏋?/span>


鍒?/span>鐢?/span>TDI鏅?/span>浣?/span>鐨?/span>鍔?/span>鑷?/span>鍙?/span>鍏?/span>鎬?/span>璐?/span>錛?/span>璇?/span>璇?/span>棰?/span>緇?/span>鎴?/span>鍔?/span>璁?/span>璁?/span>浜?/span>涓涓?/span>INHIBIT閫?/span>杈?/span>闂?/span>錛?/span>鍥?/span>5錛?/span>銆?/span>鑰?/span>姘?/span>閿?/span>浣?/span>鐢?/span>瀵?/span>鑷?/span>鐨?/span>鍙?/span>鍏?/span>棰?/span>鑹?/span>鏀?/span>鍙?/span>鍦?/span>闃?/span>浼?/span>鏍?/span>絳?/span>涓?/span>涔?/span>鏈?/span>鐫娼?/span>鍦?/span>鐨?/span>搴?/span>鐢?/span>銆?/span>濡?/span>鍥?/span>5b鎵紺?/span>錛?/span>鍦?/span>绱?/span>澶?/span>鐏?/span>涓?/span>錛?/span>MeTO/PVP鍒?/span>澶?/span>鐨?/span>鍥?/span>妗?/span>鐨?/span>棰?/span>鑹?/span>鍦?/span>姘?/span>钂?/span>姘?/span>娑?/span>婀?/span>鍓?/span>鍚?/span>鏈?/span>鐫鏄?/span>钁?/span>鐨?/span>鍙?/span>鍖?/span>銆?/span>

鍥?/span>5. INHIBIT閫?/span>杈?/span>闂?/span>鍜?/span>闃?/span>浼?/span>鏍?/span>絳?/span>


鐩?/strong>鍏?/strong>閾?/strong>鎺?/strong>

Liangwei Ma, Bingbing Ding, Zhiyi Yuan, Xiang Ma* and He Tian. Triboluminescence and Selective Hydrogen-Bond Responsiveness of Thiochromanone Derivative. ACS Mater. Lett., 2021, 3, 1300-1306.

https://pubs.acs.org/doi/10.1021/acsmaterialslett.1c00339



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